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All answers having "Harmonious" as clue:

5 Character Answers:

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ATONE

INKEY

ONKEY

TONAL



6 Character Answers:

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DULCET

INSTEP

INSYNC

INTUNE

UNITED



7 Character Answers:

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TUNEFUL



8 Character Answers:

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OFAPIECE

PLEASING



9 Character Answers:

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ACCORDANT

CONGRUENT

CONGRUOUS